subject predicate object context
9076 Creator 169f034520be3a0d0aff86e4441f6f0e
9076 Creator ext-6c219a9a6efe243b5f396e585bd54a96
9076 Date 2006-03
9076 Is Part Of repository
9076 Is Part Of p00128252
9076 abstract Uranium-series (U-series) analyses are an essential component of many research projects in Earth and environmental science, oceanography, hydrology and science-based archaeology. Topics range from magma chamber evolution and volcanic hazard prediction, global climatic change through dating of authigenic carbonate deposits, human evolution through dating of bone, to the study of groundwater evolution. The U-series decay chains contain many elements that can be fractionated in environmental and geological processes. Half-lives of radioactive isotopes of such elements range from seconds to many millennia and application depends on the natural timeframe of the process or the elapsed time. This review will be limited to some aspects of the 238U–234U–230Th–226Ra system with half-lives of 245 kyr, 76 kyr and 1.6 kyr, respectively. In environmental systems, fractionation of uranium and thorium is a very efficient process because thorium is extremely insoluble while hexavalent uranium in oxidising conditions is relatively soluble. Many authigenic precipitates of calcite contain virtually no thorium and inorganic precipitates have U/Ca ratios very similar to the ratio of dissolved uranium and calcium. Almost no radiogenic 230Th in the precipitate means that the radiogenic clock starts effectively at zero. However, pure authigenic precipitates are rare and many contain some allogenic material, mostly silicate with 238U in secular equilibrium with significant 230Th. Some of the characteristics of different types of samples and various methods to accommodate or correct for ‘inherited’ 230Th will be discussed. Authigenic material should remain a ‘closed system’ with respect to the relevant isotopes but that requirement is sometimes difficult to maintain because radioactive decay results in damage to the crystal lattice of the host mineral. Consequences of this ‘recoil effect’ and correction schemes will be discussed. Dating archaeological bone based on the systematics of diffusion and adsorption to effectively model ‘open system’ behaviour is also included.
9076 authorList authors
9076 issue 1-4
9076 status peerReviewed
9076 volume 75
9076 type AcademicArticle
9076 type Article
9076 label van Calsteren, P. and Thomas, L. (2006). Uranium-series dating applications in natural environmental science. Earth Science Reviews, 75(1-4) pp. 155–175.
9076 label van Calsteren, P. and Thomas, L. (2006). Uranium-series dating applications in natural environmental science. Earth Science Reviews, 75(1-4) pp. 155–175.
9076 Title Uranium-series dating applications in natural environmental science
9076 in dataset oro